Inhomogeneous Time-Reversal Symmetry Breaking in Sr2RuO4

We show that the observed time-reversal symmetry breaking (TRSB) of the superconducting state in Sr2RuO4 can be understood as originating from inhomogeneous strain fields near edge dislocations of the crystal. Specifically, we argue that, without strain inhomogeneities, Sr2RuO4 is a single-component, time-reversal symmetric superconductor, likely with a dx2−y2 symmetry. Due to the strong strain inhomogeneities generated by dislocations, a slowly-decaying sub-leading pairing state contributes to the condensate in significant portions of the sample. As its phase winds around the dislocation, time-reversal symmetry is locally broken. Global phase locking and TRSB occur at a sharp Ising transition that is not accompanied by a change of the single-particle gap and yields a very small heat capacity anomaly. Our model thus explains the puzzling absence of a measurable heat capacity anomaly at the TRSB transition in strained samples, and the dilute nature of the time-reversal symmetry broken state probed by muon spin rotation experiments. We propose that plastic deformations of the material may be used to manipulate the onset of broken time-reversal symmetry.